Tiger Hair is a product produced by Evercoat, and is a very high quality, expensive product that I've used many times.
It's waterproof unlike regular Bondo type body filler so it works really well if you put a little tooth (scratching) the metal so it has something to grab to.
A little lite scuffing with some 36 to 40 grit sandpaper works perfect for excellent adhesion.
Once you get the fiber strand (Tiger Hair) smoothed out by rough sanding (36-40 grit) you can skim it over with body filler, sand, prime, paint.
As far as body filler I am a 100% advocate of using Evercoat Rage Gold. It too, is not cheap, but it is superior quality and the choice of high end builders.
Time, Patience, and Quality Materials make all the difference to the end result. However, I have seen quarter panels built from paper grocery sacks and fiber strand sanded and painted.
It's not all that hard to do body work, but it will sure make a nice shop turned into a trashy shop from all the mess.
The dust will get into everything, so beware before you start.
Tom